The Sandman #12 The Doll's House P3: Playing House by Neil Gaiman
By Neil Gaiman
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39b) with two bands in the UV be assigned to pÀp* transitions of the coordinated pyridyl ring. 39 Generic structure of tris(dipicolinato)lanthanide complexes (top); (a) plot of the Ln–N (circle) and Ln–O (triangle) distances vs lanthanide ionic radius; (b) absorption spectra in water; plot of the hyperpolarisability coefficient vs ionic radius (c) or f-orbital filling (d) the absence of any ligand functionalisation suppresses the ILCT transition. The NLO activity measured in water solution is rather small, as expected for a nonfunctionalised ligand, but regularly increases along the series from lanthanum to lutetium.
50). 50 Photoswitching of the quadratic NLO response by using a photochromic metal complex 48 METAL-BASED QUADRATIC NONLINEAR OPTICAL MATERIALS PSS closed forms: the 0 value for the open form is very small, in agreement with the absence of p-conjugation between the two thiophene rings of the DTE fragment. Upon conversion to the closed form in the photostationary state, the NLO activity dramatically increased, from 160 to 1800 Â 10–48 esu. Thus, the huge enhancement of 0 clearly reflects the efficient delocalisation of the p-electron system in the closed forms and demonstrates an efficient ON/OFF switching of the NLO responses.
06 (HRS) value twice that of its neutral precursor 97 and the fully oxidised compound 972þ. Complex 97þ is a class II mixed-valence complex, retaining charge localisation, but with enough electronic coupling between the redox centres to permit intervalence charge transfer transitions. As the redox couples 97/97þ and 97þ/972þ are fully reversible, this system constitutes, like compound 95, an interesting three-states NLO switch. g. [123] They display intense visible d(FeII) ! 50 eV is observed. The difference between the two solvents may be attributed at least in part to the greater hydrogen bond donating ability of water acting to reduce the basicity and enhance the p-accepting ability of the cyanide ligands.